The bicyclo[2.{2|two}.2]diazaoctane alkaloids are a vast group of {natural|all-natural|organic} {products|goods|items|merchandise|solutions} which {have been|happen to be|have already been} the {focus|concentrate} of {attention|interest|focus|consideration} {from the|in the} scientific {community|neighborhood} for {several|a number of|numerous|many|various|quite a few} decades. This interest stems from their broad {range|variety} of biological activities, their diverse biosynthetic origins, and their topologically {complex|complicated} structures, which combined make them enticing targets for chemical synthesis. {In this|Within this} {article|post|write-up|report|short article}, {full|complete} {details|particulars|specifics|information|facts} of our synthetic {studies|research} {into the|in to the} chemical feasibility of a proposed network of biosynthetic pathways towards the brevianamide {family|family members|loved ones|household} of bicyclo[2.{2|two}.2]diazaoctane alkaloids are disclosed. Insights into {issues|problems|concerns|troubles|difficulties|challenges} of reactivity and selectivity {in the|within the|inside the} biosynthesis {of these|of those} structures have aided the {development|improvement} of a unified biomimetic synthetic {strategy|technique|method|approach|tactic}, which has resulted {in the|within the|inside the} total synthesis of all {known|recognized|identified} bicyclo[2.{2|two}.2]diazaoctane brevianamides {and the|and also the|as well as the|along with the|plus the} anticipation of an as-yet-undiscovered congener. 2-Bromo-5-(difluoromethyl)pyrazine custom synthesis 1011460-68-6 Chemscene PMID:23800738
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