Understanding and mitigating filament formation, short-circuit, and {solid|strong} electrolyte fracture {is a|is really a|is actually a|can be a|is often a|is usually a} {key|important|crucial|essential} necessity towards {achieving|reaching|attaining} {practical|sensible} SSBs. Herein, we employa coupled far-fi eld {high|higher} {energy|power} diffraction microscopy -tomography {approach|method|strategy} for assessing chemo-mechanical behavior for dense, polycrystalline garnet (Li7La3Zr2O12, LLZO) {solid|strong} electrolytes with grain-level resolution. Tracking the {stress|tension|anxiety|pressure|strain} response for individualgrains {through|via|by means of|by way of} in situ testing, failure onset and short-circuit mechanism is confirmed {to be|to become} a stochastic, isolated {process|procedure|method|approach|course of action} governed by the presence of {local|nearby|neighborhood|regional} phase heterogenity. Coupling {high|higher} {energy|power} X-ray diffraction and far eld {high|higher} {energy|power} diffraction microscopy measurements, these {local|nearby|neighborhood|regional} regions are proposed {to be|to become} regions {with the|using the|with all the|together with the} presence of acubic polymorph of LLZO arising potentially from {local|nearby|neighborhood|regional} dopant concentration variation. Interplay of mechanics and transport is evaluated and coupled tomography andFF-HEDM dataset is employed to illustrate the degradation of polycrystalline garnetsolid electrolyte. {The results|The outcomes} showcase pathways for processing {high|higher} performing SSBs. 346704-04-9 Chemscene Price of Triphenylbismuth PMID:24576999
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