This {work|function|perform|operate} reports a {process|procedure|method|approach|course of action} in which concentrated irradiation from a simulated solar {source|supply} converts methane to high-value graphitic carbon and hydrogen gas. Methane flows {within|inside} a photo-thermal reactor {through|via|by means of|by way of} the pores of a thin substrate irradiated by {several|a number of|numerous|many|various|quite a few} thousand suns {at the|in the} focal peak. The methane decomposes {primarily|mainly|mostly} into hydrogen {while|whilst|although|even though|when|though} depositing {highly|extremely|very|hugely} graphitic carbon that grows conformally {over|more than} ligaments {in the|within the|inside the} porous substrate. The localized solar heating {of the|from the|in the|on the|with the|of your} porous substrate serves to capture the {solid|strong} carbon into a readily extractable and {useful|helpful|beneficial|valuable} {form|type|kind} {while|whilst|although|even though|when|though} {maintaining|sustaining|preserving|keeping} active deposition {site|website|web site|internet site|web-site|web page} density with persistent catalytic activity. {Results|Outcomes|Final results|Benefits} indicate a {strong|powerful|robust|sturdy} temperature dependence with {high|higher} decomposition occurring {in the|within the|inside the} central heating zone with concentration {factors|elements|aspects|variables|components|things} and temperatures above 1000 suns and 1300 K, respectively. Even {with a|having a|using a} {large|big|huge|massive|substantial|significant} flow {area|region|location} {through|via|by means of|by way of} regions of {lower|reduce|reduced|decrease} irradiation and temperature, methane conversion and hydrogen yields of approx. 70\% are {achieved|accomplished}, and 58\% {of the|from the|in the|on the|with the|of your} inlet carbon is captured in graphitic {form|type|kind}. 1398507-82-8 In stock 69812-51-7 Chemscene PMID:24761411

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