{Important|Essential|Crucial|Critical|Significant|Vital} efforts are {currently|presently|at present|at the moment} {under|below|beneath} way {in order to|to be able to|as a way to|in an effort to|so as to|so that you can} implement plasmonic phenomena {in the|within the|inside the} {growing|expanding|developing|increasing} field of photocatalysis, striving for {improved|enhanced} efficiency and reaction selectivity. A {significant|substantial|considerable|important} fraction of such efforts has been focused on distinguishing, understanding and enhancing {specific|particular|certain|distinct|precise} {energy|power} transfer mechanisms from plasmonic nanostructures to their {environment|atmosphere}. Herein we report a synthetic {strategy|technique|method|approach|tactic} that brings {together|with each other|collectively} two {of the|from the|in the|on the|with the|of your} {main|primary|principal|major|key|most important} physical mechanisms driving plasmonic photocatalysis into an engineered {system|method|program|technique} by rationally combining the photochemical {features|attributes|functions|characteristics|capabilities|options} of energetic charge carriers {and the|and also the|as well as the|along with the|plus the} electromagnetic field enhancement inherent {to the|towards the|for the} plasmonic excitation. We do so by {creating|making|producing|generating|developing|building} hybrid photocatalysts that integrate {multiple|numerous|several|a number of|many|various} plasmonic resonators {in a|inside a|within a} single entity, controlling their joint contribution {through|via|by means of|by way of} spectral separation and differential surface functionalization. This {strategy|technique|method|approach|tactic} {allows|enables|permits|makes it possible for} us to study the {combination|mixture} of {different|various|distinct|diverse|unique|distinctive} photosensitization mechanisms when activated simultaneously. Our {results|outcomes|final results|benefits} show that hot electron injection {can be|may be|could be|might be|is often|is usually} combined with an {energy|power} transfer {process|procedure|method|approach|course of action} mediated by near-field interaction, {leading|top|major} to a {significant|substantial|considerable|important} {increase|improve|boost|enhance|raise} {of the|from the|in the|on the|with the|of your} final photocatalytic response {of the|from the|in the|on the|with the|of your} material. {In this|Within this} manner, we overcome the limitations that hinder photocatalysis driven only by a single {energy|power} transfer mechanism, and move the field of plasmonic photocatalysis closer to energy-efficient applications. {Furthermore|Moreover|In addition|Additionally}, our multimodal hybrids {offer|provide|supply|offer you|present|give} a test {system|method|program|technique} to probe the properties {of the|from the|in the|on the|with the|of your} two targeted mechanisms in energy-related applications {such as|like|including|for example|for instance|which include} the photocatalytic generation of hydrogen and open the door to wavelength-selective photocatalysis and novel tandem reactions. Boc-Ser-OtBu Chemical name 3-Hydroxy-5-methoxybenzaldehyde structure PMID:24140575
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