CO2 valorization is aimed at converting waste CO2 to value-added {products|goods|items|merchandise|solutions}. {While|Whilst|Although|Even though|When|Though} steady progress has been {achieved|accomplished} {through|via|by means of|by way of} diverse catalytic {strategies|methods|techniques|approaches|tactics}, {including|such as|which includes|like} CO2 electrosynthesis, CO2 thermocatalysis, and biological CO2 fixation, {each|every|each and every|every single} {of these|of those} approaches have distinct limitations. Inorganic catalysts only {enable|allow} synthesis beyond C2 and C3 {products|goods|items|merchandise|solutions} with poor selectivity and {with a|having a|using a} {high|higher} {energy|power} requirement. Meanwhile, {although|even though|though|despite the fact that|while} biological organisms can selectively {produce|create|generate|make} {complex|complicated} {products|goods|items|merchandise|solutions} from CO2, their slow autotrophic metabolism limits their industrial feasibility. {Here|Right here}, we present an abiotic {approach|method|strategy} leveraging electrochemical and thermochemical catalysis {to complete|to finish} the conversion of CO2 to life-sustaining carbohydrate sugars akin to photosynthesis. CO2 was electrochemically converted to glycolaldehyde and formaldehyde {using|utilizing|making use of|employing|working with|applying} copper nanoparticles and boron-doped diamond cathodes, respectively. CO2-derived glycolaldehyde then served {as the|because the} {key|important|crucial|essential} autocatalyst for the formose reaction, {where|exactly where} glycolaldehyde and formaldehyde combined {in the|within the|inside the} presence of an alkaline earth metal catalyst to {form|type|kind} {a variety of|a number of|many different|various|a range of|several different} C4 – C8 sugars, {including|such as|which includes|like} glucose. In turn, these sugars {were|had been|have been} {used|utilized|employed|utilised|applied|made use of} as a feedstock for fast-growing and genetically modifiable Escherichia coli. Altogether, {we have|we’ve|we’ve got} assembled a platform that pushes the boundaries of {product|item|solution} complexity achievable from CO2 conversion {while|whilst|although|even though|when|though} demonstrating CO2 integration into life-sustaining sugars. 1934533-59-1 Chemscene 6-Bromo-2,3-dihydrobenzofuran site PMID:24238102
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