The synthesis of bottlebrush polymers with topologically precise and {fully|totally|completely} discrete structures is reported. {Key|Important|Crucial|Essential} {features|attributes|functions|characteristics|capabilities|options} {of the|from the|in the|on the|with the|of your} synthesis {include|consist of|contain|incorporate|include things like|involve} the {combination|mixture} of scalable synthesis and separation {strategies|methods|techniques|approaches|tactics} to access discrete macromonomer libraries, followed by their polymerization and {further|additional} separation into topologically uniform and discrete bottlebrushes. Discrete macromonomers prove {crucial|essential|vital|critical|important} for regulating the structural heterogeneity of bottlebrushes and their macroscopic properties. When assembled as a monolayer {at the|in the} air-water interface, bottlebrushes with discrete side chains {display|show} {high|higher} packing density and distinct three-phase Langmuir-Blodgett isotherms. The {impact|influence|effect} of precisely regulating side chain dispersity and sequence on polymer properties was {further|additional} demonstrated {through|via|by means of|by way of} tailoring the interbrush interactions and thermomechanical properties of well-defined block bottlebrushes. Formula of 259214-55-6 106-86-5 supplier PMID:35670838
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