The diverse optical, magnetic, and electronic behaviors of most colloidal semiconductor nanocrystals emerge from {materials|supplies|components} with {limited|restricted} structural and elemental compositions. Conductive metal-organic frameworks (MOFs) possess {rich|wealthy} compositions with {complex|complicated} architectures, but {remain|stay} unexplored as nanocrystals, hindering their incorporation into scalable devices. {Here|Right here}, we report the controllable synthesis of conductive MOF nanoparticles {based|primarily based} on Fe(1,{2|two},3-trizolate){2|two}. Sizes {can be|may be|could be|might be|is often|is usually} tuned as {small|little|tiny|modest|smaller|compact} as {5|five}.{5|five} nm, {ensuring|making certain|guaranteeing|making sure} indefinite colloidal stability. These solution-processable MOFs {can be|may be|could be|might be|is often|is usually} analyzed by solution-state spectroscopy and electrochemistry and cast into conductive thin films with {excellent|superb|outstanding|exceptional|great|fantastic} uniformity. This unprecedented {analysis|evaluation} of MOF {materials|supplies|components} reveals a {strong|powerful|robust|sturdy} size-dependence in optical and electronic behavior sensitive {to the|towards the|for the} intrinsic porosity and guest-host interactions of MOFs. These {results|outcomes|final results|benefits} {provide|offer|supply|give|present|deliver} a radical departure from {typical|common|standard} MOF characterization, enabling insight into physical properties otherwise {impossible|not possible} with bulk analogs, {while|whilst|although|even though|when|though} {offering|providing|supplying} a roadmap for the future of MOF nanoparticle synthesis and device fabrication. tert-Butyl 3-bromopropanoate Purity Iridium(III) chloride xhydrate site PMID:35567400
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