The synthesis of nanohoop rotaxanes {via|by way of|through|by means of} twodifferent active template {strategies|methods|techniques|approaches|tactics} is reported. By preparingtriazole-embedded rotaxanes, the observation of metal binding events in bothorganic and aqueous {conditions|circumstances|situations} are readily observed {via|by way of|through|by means of} dramatic {changes|modifications|adjustments|alterations} innanohoop emission. Inspired by this {result|outcome}, we then describe the designand synthesis of {a new|a brand new} {type|kind|sort|variety|form} of “self-destructing” nanohoop rotaxanethat, {in the|within the|inside the} presence of an analyte, releases a quenched nanohoop macrocycleresulting {in a|inside a|within a} {bright|vibrant} fluorescence response. Morebroadly, this {work|function|perform|operate} highlights the conceptual {advantages|benefits|positive aspects} of combining compact π-rich macrocyclic frameworks withmechanical bonds formed {via|by way of|through|by means of} active-template syntheses. 2-Bromo-N-phenylaniline custom synthesis 335357-38-5 custom synthesis PMID:23551549
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