This {work|function|perform|operate} elaborates the {effect|impact} of dynamic irradiation on light-driven molecular water oxidation to counteract catalyst deactivation. It highlights the {importance|significance|value} of {overall|general|all round} reaction engineering to overcome limiting {factors|elements|aspects|variables|components|things} in artificial photosynthesis reactions. Systematic investigation of a homogenous {three|3} {component|element} ruthenium-based water oxidation {system|method|program|technique} revealed {significant|substantial|considerable|important} {potential|possible|prospective} to {enhance|improve|boost} the {overall|general|all round} catalytic efficiency by synchronizing the timescales of photoreaction and mass transport {in a|inside a|within a} capillary flow reactor. The {overall|general|all round} activity {could be|might be|could possibly be|may be|may very well be} {improved|enhanced} by a {factor|aspect|element|issue} of {more|much more|a lot more|far more|additional|extra} than {10|ten} with respect {to the|towards the|for the} turnover {number|quantity} {and a|along with a|as well as a|plus a|and also a|in addition to a} {factor|aspect|element|issue} of 31 referring {to the|towards the|for the} external {energy|power} efficiency by controlling the {local|nearby|neighborhood|regional} availability of photons. Detailed insights {into the|in to the} mechanism of light driven water oxidation {could be|might be|could possibly be|may be|may very well be} obtained {using|utilizing|making use of|employing|working with|applying} complementary {methods|techniques|strategies|approaches|procedures|solutions} of investigation like Raman, IR and UV-vis/emission spectroscopy, unraveling the {importance|significance|value} of avoiding {high|higher} concentrations of excited photosensitizers. 224295-73-2 In stock BuyTrifluoromethanesulfonic acid (silver) PMID:24211511
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